Magnetic behavior of yavapaiite-type BaMoP2O8 with the spatially anisotropic triangular arrangement of the S = 1 Mo 4+ ions is explored using thermodynamic measurements, neutron diffraction, and density-functional band-structure calculations. A broad maximum in the magnetic susceptibility around 46 K is followed by the stripe antiferromagnetic order with the propagation vector k = ( 1 2 , 1 2 , 1 2 ) formed below TN 21 K. This stripe phase is triggered by a pronounced onedimensionality of the spin lattice, where one of the in-plane couplings, J2 4.6 meV, is much stronger than its J1 0.4 meV counterpart, and stabilized by the weak easy-axis anisotropy. The ordered moment of 1.42(9) µB at 1.5 K is significantly lower than the spin-only moment of 2 µB due to a combined effect of quantum fluctuations and spin-orbit coupling.