2024
DOI: 10.1002/cctc.202301399
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One‐Pot N‐Alkylation of Amines over Ni(II) Embedded Reusable Porous Organic Polymer via Borrowing Hydrogen Strategy

Debabrat Pathak,
Bikash Kumar Kalita,
Himanshu Sharma
et al.

Abstract: The first‐of‐its‐kind, one‐pot N‐alkylation reaction of amines over Ni(II) impregnated porous organic polymer of highly dense N‐rich skeleton is reported. The primeval Ni(II) decorated hollow spherical porous polymer is synthesized and employed in a series of catalytic reactions involving C–N bond formation. The catalytic reactions are optimised to yield the desired product highlighting the role of different substituents present on the reactants towards the overall selectivity and efficiency. The detailed reac… Show more

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