2021
DOI: 10.1039/d1ta01267c
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One-step fabrication of a laser-induced forward transfer graphene/CuxO nanocomposite-based electrocatalyst to promote hydrogen evolution reaction

Abstract: Electrochemical water splitting is an attractive strategy to realize hydrogen harvesting. Exploring highly efficient electrocatalysts based non-precious material is of great significance to break the dilemma of noble metal-based materials...

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Cited by 26 publications
(14 citation statements)
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“…Obviously, the required η at 300 mA cm –2 for the IO/CP/CF (298 mV) is much smaller in comparison with the Pt/C–CF (406 mV). The HER activity of IO/CP/CF is also superior to the Cu-based electrocatalysts reported recently, for instance, the alloyed Cu–Ni nanocage, Ag@Cu 2 O/CF, and LIFT graphene/Cu x O@Ni foam . In Figure b, the Tafel slopes of IO/CF, CP/CF, IO/CP/CF, and Pt/C–CF are respectively 112, 91, 73, and 77 mV dec –1 , proposing the Volmer–Heyrovsky pathway toward HER .…”
Section: Resultsmentioning
confidence: 63%
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“…Obviously, the required η at 300 mA cm –2 for the IO/CP/CF (298 mV) is much smaller in comparison with the Pt/C–CF (406 mV). The HER activity of IO/CP/CF is also superior to the Cu-based electrocatalysts reported recently, for instance, the alloyed Cu–Ni nanocage, Ag@Cu 2 O/CF, and LIFT graphene/Cu x O@Ni foam . In Figure b, the Tafel slopes of IO/CF, CP/CF, IO/CP/CF, and Pt/C–CF are respectively 112, 91, 73, and 77 mV dec –1 , proposing the Volmer–Heyrovsky pathway toward HER .…”
Section: Resultsmentioning
confidence: 63%
“…The HER activity of IO/CP/CF is also superior to the Cu-based electrocatalysts reported recently, for instance, the alloyed Cu−Ni nanocage, 11 Ag@Cu 2 O/CF, 13 and LIFT graphene/Cu x O@Ni foam. 46 In Figure 3b, the Tafel slopes of IO/CF, CP/CF, IO/CP/CF, and Pt/C−CF are respectively 112, 91, 73, and 77 mV dec −1 , proposing the Volmer− Heyrovsky pathway toward HER. 13 The IO/CP/CF with a lower Tafel slope demonstrates its improved water dissociation kinetics.…”
Section: Resultsmentioning
confidence: 88%
“…28,29 This variant of LIG boasts exceptional conductivity and catalytic activity, making it ideal for efficient power generation in microbial fuel cells (MFCs) and presenting a scalable alternative to costly catalysts like platinum. 30,31 The laser-based production technique ensures high-purity graphene with outstanding structural integrity, allowing versatile use of carbon sources, precise property control, and integration into existing manufacturing processes. 28,32 Its rapid and cost-efficient graphene production has led to applications across diverse fields like energy storage, electrocatalysis, water treatment, and sensing due to its unmatched physicochemical properties.…”
Section: ■ Introductionmentioning
confidence: 99%
“…Laser-induced graphene (LIG) represents a distinctive layered form of graphene generated on polymer-based carbonous substrates using a CO 2 laser, offering a reagent-free and straightforward method for graphene production. , Undergoing sulfur doping through poly­(ether sulfone) (PES) results in sulfur-doped LIG, showcasing superior electrocatalytic properties attributed to heightened charge storage and the creation of more active catalytic sites via carbon–sulfur interactions. , This variant of LIG boasts exceptional conductivity and catalytic activity, making it ideal for efficient power generation in microbial fuel cells (MFCs) and presenting a scalable alternative to costly catalysts like platinum. , The laser-based production technique ensures high-purity graphene with outstanding structural integrity, allowing versatile use of carbon sources, precise property control, and integration into existing manufacturing processes. , Its rapid and cost-efficient graphene production has led to applications across diverse fields like energy storage, electrocatalysis, water treatment, and sensing due to its unmatched physicochemical properties . Notably, LIG’s antiviral, antibacterial, and antibiofouling attributes make it pertinent in energy, environmental, and biomedical domains .…”
Section: Introductionmentioning
confidence: 99%
“…It is worth noticing the traditional methods to fabricate graphene are commonly complicated and expensive. Laser direct writing method from portable carbon precursors to fabricate graphene is a potential approach to promote and expand the graphene application in different fields, like supercapacity, electrocatalysts, photothermal sterilization and wearable devices [15][16][17][18][19].…”
Section: Introductionmentioning
confidence: 99%