“…In addition, some studies used carbon isotope dating to differentiate contributions from biomass burning to fossil fuel combustion (Mandalakis et al, 2005; Sheesley et al, 2009; Zencak et al, 2007). While the molecular diagnostic ratio (MDR) technique has been applied in several studies (Fu et al, 2010; Schifman and Boving, 2015; Zhang et al, 2005), many PAH MDRs vary significantly in space and time due to different reaction rates in the atmosphere and the estimates were not valid source markers (Amador-Munoz et al, 2013; Katsoyiannis et al, 2011; Tobiszewski and Namiesnik, 2012). Major sources identified as contributing to ambient PAH concentrations include open burning of agriculture residuals (Chen et al, 2008), gasoline and diesel vehicles (Larsen and Baker, 2003), coal combustion (Chen et al, 2011), wood combustion (Piazzalunga et al, 2013) and industrial sources such as refineries (Motelay-Massei et al, 2007).…”