1999
DOI: 10.1063/1.124086
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Optical nonlinearity in low-temperature-grown GaAs: Microscopic limitations and optimization strategies

Abstract: We have quantitatively measured the linear and the nonsaturable absorption as well as the absorption modulation and its recovery time in as-grown and annealed low-temperature (LT) GaAs. Correlation of the optical data with As antisite (AsGa) defect densities yields the absorption cross section and the saturation parameter of the dominant AsGa to the conduction-band defect transition. We show that this defect transition is mainly responsible for the large nonsaturable absorption in as-grown LT GaAs with fast re… Show more

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Cited by 61 publications
(38 citation statements)
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“…In Figure 12b, we plot the characteristic decay time to 1/e (τ 1/e ) as a function of QW growth temperature. The observed behavior confirms previous studies carried out with LT-grown GaAs [52]. Although the parameter τ 1/e is not sufficient to fully characterize the dynamics of the absorber, it is an appropriate simplified parameter to compare the recovery of the absorber in a passively modelocked solid-state laser.…”
Section:  Resultssupporting
confidence: 86%
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“…In Figure 12b, we plot the characteristic decay time to 1/e (τ 1/e ) as a function of QW growth temperature. The observed behavior confirms previous studies carried out with LT-grown GaAs [52]. Although the parameter τ 1/e is not sufficient to fully characterize the dynamics of the absorber, it is an appropriate simplified parameter to compare the recovery of the absorber in a passively modelocked solid-state laser.…”
Section:  Resultssupporting
confidence: 86%
“…In Figure 12a, pump-probe measurements of these samples are shown, confirming as expected that samples grown at lower temperatures have faster recovery times [52]. In Figure 12b, we plot the characteristic decay time to 1/e (τ 1/e ) as a function of QW growth temperature.…”
Section:  Resultssupporting
confidence: 79%
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“…Their fabrication involves molecular beam epitaxy (MBE) 6 . To reduce the relaxation time to sub-picosecond levels, either postgrowth ion-implantation or low-temperature growth is normally required 6,17 . Furthermore, SESAMs are based on a resonant nonlinearity, which tends to limit wavelength tuneability 18,19 for the shortest pulse lasers 20 .…”
mentioning
confidence: 99%
“…Therefore, defects have to be introduced to the material to provide additional defect states for faster carrier trapping. Methods to obtain fast saturable absorber materials are lowtemperature (LT) growth by molecular beam epitaxy and ion implantation [10]. However, GaAs epitaxially grown on CaF 2 already provides high defect concentration at typical growth temperatures due to lattice-mismatched growth.…”
Section: Discussionmentioning
confidence: 99%