Spectral broadening is desirable in optical parametric oscillators (OPOs) for their tunability and generation of short pulses, which typically entails more complex systems and increased costs. Here, we report large-scale spectral broadening through the simple insertion of a MoTe 2 film into the cavity of a femtosecond OPO for the first time. The OPO offers a tunable output ranging from 1245 to 1552 nm, and comparable broadening effects are observed in most of the operating wavelengths. The broadest spectrum is achieved at 1524 nm by inserting a lowconcentration 1T′-MoTe 2 film, exhibiting a spectral broadening factor exceeding 22. Spectral broadening results in a time compression correspondingly. The narrowest pulse is obtained by using a low-concentration 2H-MoTe 2 film with a pulse duration of 88 fs, and a temporal compression of 20 of pulse duration is obtained at 1417 nm. The experimental results show that the nonlinear properties and the film structure of MoTe 2 induce a local modulation of the signal in the space−time domain, representing the main contribution to spectral broadening. This approach will offer new insights to enhance the practical application of 2D materials and benefit the development of OPO devices.