deep sea, underground, chemical plants, environmental disasters areas, and agricultural farmland. [7] Radio frequency energy harvesting (RFEH) has emerged as a promising option for powering IoTbased devices due to the broad availability of radio frequency (RF) signals, which, despite their relatively low energy density, are accessible in places where other energy sources such as solar and thermal energy are unavailable or limited. [8][9][10] However, conventional RFEH systems have limitations in terms of their cost, size, weight, and foldability. As a result, many studies have attempted to combine novel fabrication methods and ambient RFEH to produce low-cost, light, small, and foldable power supply systems. [11][12][13][14] Cellulose paper is a promising substrate for the fabrication of RFEH systems that satisfy these requirements. Paper has recently gained significant attention as a component of electronics due to its abundance, disposability, recyclability, biocompatibility, light weight, cost-effectiveness, and flexibility. [15][16][17] Based on these advantages, paper or paper-like substrates have been utilized in a variety of applications ranging from basic electronic units to complicated electronic devices such as supercapacitors (SCs), [18,19] light-emitting diodes (LEDs), [20] transistors, [21] biofuel cells, [22] RF antenna, [23] and sensors. [24] However, it remains difficult to employ conventional methods for the fabrication of paper-based electronics in the development of integrated foldable RFEH systems that incorporate an RF antenna, RF/direct current (DC) rectifier, and energy storage unit. The main reason for this is the limitations associated with paper when seeking to fabricate a stable electrode due to its high porosity, hygroscopy, and surface roughness. [15] In general, the porosity and surface roughness of a substrate are important properties affecting the quality of a fabricated electrode because they can affect ink or particle penetration continuity and disrupt conductive paths if they are too high. [25] As a result, the roughness and porosity of paper substrates for electronic applications need to be reduced. [26,27] In particular, because RF electronics require a more stable and homogeneous substrate and higher conductivity than DC components, [28,29] untreated paper is generally not suitable for RF electronics. In addition, the hygroscopic nature of conventional paper hinders the complicated patterning required for RF electronics, such as the fabrication of uniform micro-sized lines, vias, and conductive patterning on both sides of paper. Radio frequency energy harvesting (RFEH) systems have emerged as a critical component for powering devices and replacing traditional batteries, with paper being one of the most promising substrates for use in flexible RFEH systems. However, previous paper-based electronics with optimized porosity, surface roughness, and hygroscopicity still face limitations in terms of the development of integrated foldable RFEH systems within a single sheet of paper....