This study improved the performances of a thin-film transistor (TFT) device with n-type Ti-doped GaZnO (GTZO) as the channel layer. Various O 2 /Ar ratios were used during radio-frequency magnetron sputtering deposition to modify the carrier concentration and the thin-film surface flatness. Atomic force microscopy results indicate that the lowest surface roughness (0.38 nm) was observed in the GTZO films fabricated at an O 2 /Ar ratio of 12/30 sccm. In addition, a room-temperature X-ray diffraction and photoluminescence study verified the improved crystal quality and decreased oxygen vacancies as the O 2 /Ar ratio increased. The GTZO films fabricated at an O 2 /Ar gas flow of 6/30 sccm were adopted as the transistor channel layer of a TFT, which exhibited an improved carrier mobility of 16.1 cm 2 V À1 s À1 , a subthreshold swing of 0.43 V dec À1 , an off current of 5.6 Â 10 À13 A, and an on-off current ratio of 2.2 Â 10 8 . From the comparison of transfer characteristic curves for the TFTs with channels of ZnO, indium gallium zinc oxide, and GTZO in this study, the GTZO TFTs exhibit superior characteristics which demonstrated the potential for high-performance optoelectronic device applications.