Metasurfaces are opening promising flexibilities to reshape the wavefront of electromagnetic waves. Notable optical phenomena are observed with the tailored surface plasmon, which is excited by metallic components in the visible spectrum. However, metamaterial or metasurface devices utilizing metallic materials encounter the challenge of low transmission efficiency, particularly within the visible spectrum. This study proposes a multilayer design strategy to enhance their transmission efficiency. By incorporating additional metal layers for improvements in the transmission efficiency and dielectric layers as spacers, cavities are formed along the propagation direction, enabling the modulation of transmittance and reflection through a process mimicking destructive interference. An analytical model simplified with the assumption of deep-subwavelength-thick metal layers is proposed to predict the structural parameters with optimized transmittance. Numerical studies employing the rigorous coupled wave analysis method confirmed that the additional metal layers significantly improve the transmittance. The introduction of the extra metal and dielectric layers enhances the transmission efficiency in specific spectral regions, maintaining a controllable passband and transmittance. The results indicate that the precise control over the layers’ thicknesses facilitates the modulation of peak-to-valley ratios and the creation of comb-like filters, which can be further refined through controlled random variation in the thickness. Furthermore, when the thickness of the silver layer followed an arithmetic sequence, a multilayer structure with a transmittance of approximately 80% covering the entire visible spectrum could be achieved. Significantly, the polarization extinction ratio and the phase delay of the incident beams could still be modulated by adjusting the geometrical structure and parameters of the multilayer metamaterial for diversified functionalities.