2024
DOI: 10.1002/ange.202319029
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Optimizing Intermediate Adsorption over PdM (M=Fe, Co, Ni, Cu) Bimetallene for Boosted Nitrate Electroreduction to Ammonia

Yuanbo Zhou,
Lifang Zhang,
Zebin Zhu
et al.

Abstract: Electrochemical reduction of nitrate to ammonia (NO3RR) is a promising and eco‐friendly strategy for ammonia production. However, the sluggish kinetics of the eight‐electron transfer process and poor mechanistic understanding strongly impedes its application. To unveil the internal laws, herein, a library of Pd‐based bimetallene with various transition metal dopants (PdM (M=Fe, Co, Ni, Cu)) are screened to learn their structure‐activity relationship towards NO3RR. The ultra‐thin structure of metallene greatly … Show more

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