2024
DOI: 10.1021/acs.joc.4c00131
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Organocatalytic Dearomative Spirocyclization Reaction of Enone-Tethered α-and β-Naphthols and Dearomatization Reaction of In Situ Generated Nitro-Olefin-Tethered α-Naphthols

Amit Shikari,
Madhur Sharma,
Kalishankar Bhattacharyya
et al.

Abstract: Herein, we report a catalytic dearomative spirocyclization reaction of new substrates having aryl/alkyl enone tethered αand β-naphthols and a dearomatization reaction of in situ generated nitro-olefin-tethered α-naphthols. The spirocarbocycles were obtained in moderate to good yields with high diastereoselectivities. A preliminary catalytic asymmetric variant was reported. A few applications such as hydrogenations and epoxidation reaction have also been demonstrated. Theoretical study has also been performed t… Show more

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