“…Electrochemical energy technologies, including various types of batteries, fuel cells, solar cells, and supercapacitors, are considered to be one of the most reliable, efficient, and environmentally friendly methods for energy storage and conversion. , Among them, supercapacitors, characterized by high power density, fast charge–discharge rate, and long cycle life, have attracted much attention. Unfortunately, the energy density of currently available supercapacitors is significantly lower than those of full cells and batteries. , Because the electrostatic charge accumulated in the electrode/electrolyte interface has positive effects on the specific capacitance of supercapacitors, the design and optimization of electrode material are thus supposed to increase the energy density. A large number of materials including carbon materials, metal oxides, and polymers have been investigated for the electrodes in recent years, among which the carbon materials have high potential because of their low cost, good recyclability, and structural controllability. − …”