The impact of doping In 2 Se 3 in Sb thin films on the crystal structure and electrical properties was investigated. The results demonstrate that the incorporation of In 2 Se 3 enhances the thermal stability and the data retention properties of the film. Moreover, it effectively mitigates resistance drift and elevates the band gap of Sb films. Appropriate doping with In 2 Se 3 inhibits grain growth, refines grain size, and facilitates the formation of an In−Sb bond. Additionally, surface roughness is reduced upon introduction of In 2 Se 3 into Sb, leading to significantly enhanced adhesion between the film and substrate, thereby improving device reliability.