Cosmic ray muons passing through matter lose energy from inelastic collisions with electrons and are deflected from nuclei due to multiple Coulomb scattering. The strong dependence of scattering on atomic number Z and the recent developments on position sensitive muon detectors indicate that multiple Coulomb scattering could be an excellent candidate for spent nuclear fuel imaging. Muons present significant advantages over existing monitoring and imaging techniques and can play a central role in monitoring nuclear waste and spent nuclear fuel stored in dense well shielded containers. The main purpose of this paper is to investigate the applicability of multiple Coulomb scattering for imaging of spent nuclear fuel dry casks stored within vertical and horizontal commercial storage dry casks. Calculations of muon scattering were performed for various scenarios, including vertical and horizontal fully loaded dry casks, half loaded dry casks, dry casks with one row of fuel assemblies missing, dry casks with one fuel assembly missing and empty dry casks. Various detector sizes (1.2 m x 1.2 m, 2.4 m x 2.4 m and 3.6 m x 3.6 m) and number of muons (10 5 , 5·10 5 , 10 6 and 10 7 ) were used to assess the effect on image resolution. The Point-of-Closest-Approach (PoCA) algorithm was used for the reconstruction of the stored contents. The results demonstrate that multiple Coulomb scattering can be used to successfully reconstruct the dry cask contents and allow identification of all scenarios with the exception of one fuel assembly missing. In this case, an indication exists that a fuel assembly is not present; however the resolution of the imaging algorithm was not enough to identify exact location.*Corresponding author: schatzid@purdue.edu
I. INTRODUCTIONSince the pioneering work of E.P. George [1] and L. Alvarez [2], relativistic muons have been shown to have the ability to penetrate dense materials and by monitoring the subsequent scattering and/or attenuation of muons, a measurable signal about the structure and composition of the interrogated material can be obtained [3]. Recently, cosmic ray muons have been investigated for volcano imaging and cargo scanning applications and their use has been extended to nuclear waste imaging and determination of molten nuclear fuel location in nuclear reactors having suffered from the effects of a severe accident similar to the one happened in Fukushima [4][5][6][7][8][9][10][11][12][13][14][15][16][17][18][19][20][21][22][23].Earlier muon radiographic techniques were based on attenuation principles. A new promising method based on multiple Coulomb scattering was developed and demonstrated at LANL for detection of high-Z materials hidden in a large volume of low-Z materials, a situation representative of shielded material shielded hidden in a cargo container [24,25]. It was suggested that muon momentum measurement which can be achieved by indirectly measuring muon scattering in several layers of materials with known thickness could improve image resolution.This was later demonstrate...