2023
DOI: 10.1021/acsanm.3c01540
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Pd Nanoparticles Supported on N-Incorporated Hybrid Organosilica as an Active and Selective Low-Temperature Phenol Hydrogenation Catalyst

Abstract: A heterogeneous Pd-NPMO hybrid-silica catalyst is synthesized and its application for aqueous phase selective hydrogenation of phenol to cyclohexanone at near ambient temperature (40 °C) and under atmospheric hydrogen pressure is demonstrated. The homogeneously distributed Pd nanoparticles on N-bridged hybrid mesoporous organosilica showed remarkable activity and selectivity for cyclohexanone compared to the unmodified Pd-SBA-15 catalyst. Control experiments strongly claim the role of nitrogen domains in the o… Show more

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