Perovskite–organic tandem solar cells with indium oxide interconnect

Brinkmann, Kai Oliver; Becker, Tim; Zimmermann, Florian; Kreusel, Cedric; Gahlmann, Tobias; Theisen, Manuel; Haeger, Tobias; Olthof, Selina; Tückmantel, Christian; Günster, Manuel; Maschwitz, Timo; Göbelsmann, Fabian; Koch, Christine; Hertel, Dirk; Caprioglio, Pietro; Peña‐Camargo, Francisco; Perdigón‐Toro, Lorena; Al‐Ashouri, Amran; Merten, Lena; Hinderhofer, Alexander; Gomell, Leonie; Zhang, Siyuan; Schreiber, Frank; Albrecht, Steve; Meerholz, Klaus; Neher, Dieter; Stolterfoht, Martin; Riedl, Thomas

doi:10.1038/s41586-022-04455-0

Cited by 272 publications

(252 citation statements)

References 58 publications

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“…29 Very recently, a highly efficient interconnect based on an ultrathin ALD-grown InO x layer with a thickness of only about 1.5 nm was developed for perovskite-organic tandem cells. 54 As such, the low-temperature ALD technique was used to shed light on the improved deposition of TCO-based RLs for future use in all-PTSCs.…”

Section: State-of-the-art Icls In All-ptscsmentioning

confidence: 99%

Efficient interconnecting layers in monolithic all-perovskite tandem solar cells

Zhang

Lin

2022

Energy Environ. Sci.

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Section: State-of-the-art Icls In All-ptscsmentioning

confidence: 99%

Efficient interconnecting layers in monolithic all-perovskite tandem solar cells

Zhang

Lin

2022

Energy Environ. Sci.

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“…[146] Practically, the restriction of the number of junctions to twojunction SC devices could enable benefits in terms of minimized technological complexity, high-efficiency, and low-cost potentials. [278] As illustrated in Figure 5g, a wide range of material combinations have been developed in two junctions tandem PV technologies such as III-Vs, [146] III-V/Si [279][280][281] (PCE best = 35,9%), [280] perovskite/Si [282][283][284] (PCE best = 29.8%), [13] chalcogenide/Si, [278] perovskite/perovskite [285][286][287] (PCE best = 26,4%), [288] perovskite/ CIGS [289][290][291] (PCE best = 25%), [290] perovskite/organic [292,293] (PCE best = 24%), [294] organic/organic [295,296] (PCE best = 20.2%), [297] a-Si/organic (PCE best = 15.1%), [298] and many others. [51] Several research works addressed a generalized guide for the theoretical maximum PCE of two-junction tandem configuration as a function of top and bottom sub-cell bandgaps with both 2-terminal and 4-terminal architectures.…”

Section: Bandgap Tuning In Multijunction Sc Technologies With Tandem ...mentioning

confidence: 99%

“…The corresponding system combined a wide‐gap (1.85 eV) perovskite FA 0.8 Cs 0.2 Pb(I 0.5 Br 0.5 ) 3 subcell with narrow‐gap (1.33 eV) PM6:Y6 organic subcell featuring non‐fullerene acceptors. [ 294 ] Impressively, tandem organic technology enabled a breakthrough in the field of OSC by entering the era of 20% efficiency.…”

Section: State Of the Art Of Tunable Solar Cell Technologiesmentioning

confidence: 99%

Tunable Photovoltaics: Adapting Solar Cell Technologies to Versatile Applications

Meddeb

Götz‐Köhler

Neugebohrn

et al. 2022

Advanced Energy Materials

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solar, wind, hydro, geothermal, and biomass, to enable a steady mitigation of greenhouse gas emissions, which are causing the planetary climate change and global warming. [5][6][7] Additionally, due to the economic development and the worldwide urbanization, a continuous rise of the global energy consumption across all key sectors, that is, power, heating, industry, and transport is occurring. This is expressed by an increase in the annual global electricity demand by 4.5% in 2021 corresponding to additional 1000 TWh. [4] Hence, strict criteria for the selection of competitive and abundant energy alternatives are imposed, requiring high yield at affordable prices. [8] The share of total renewables power generation excluding hydropower exceeded 3000 TWh in 2020, corresponding to almost 12% of the global electricity generation. [3] Considering an effective synergy between various sustainable energy candidates, solar photovoltaics (PV) have demonstrated great capabilities that can satisfy the requirements in the pathway towards 100% renewable electricity. [9][10][11][12] Owing to the research and development activities over the last decades, the power conversion efficiencies of solar cells (SC) have skyrocketed with a prolonged operation lifetime (>15 years) and a drastic plummeting in manufacturing costs (global average module selling price below $0.25 per W). [6,[13][14][15] The rapid universal deployment of PV resulted in a contribution of about 3.4% in the worldwide electricity generation in 2020. [3] Presently, the global installed PV capacity is approaching 1 TW and it is envisioned to reach ≈10 TW by 2030 and 30 to 70 TW by 2050. [16] Interestingly, along with massive electricity production using conventional solar power plants and rooftop solar panels, ancillary concepts of PV offer new strategies for supplying modern systems in versatile applications. [17][18][19] Moreover, diverse functionalities beyond solar energy harvesting can be afforded by adaptive PV, including aesthetic appearance, visual comfort and thermal management. [17,18,20,21] The distributed nature and the ubiquitous accessibility of multifunctional PV products are substantial features of solar PV in contrast to other renewable energies. However, traditional SCs dominating the market impose intrinsic optoelectronic and thermomechanical limitations, that prohibit their multifunctional utilization. To overcome these drawbacks, novel functional materials and innovative device architecture Solar photovoltaics (PV) offer viable and sustainable solutions to satisfy the growing energy demand and to meet the pressing climate targets. The deployment of conventional PV technologies is one of the major contributors of the ongoing energy transition in electricity power sector. However, the diversity of PV paradigms can open different opportunities for supplying modern systems in a wide range of terrestrial, marine, and aerospace applications. Such ubiquitous and versatile applications necessitate the development of PV technologies with customized desig...

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“…The PCE increased and reached a maximum value at about 25 h. This "burn-in" behavior has been previously noted as a characteristic of p-i-n perovskite solar cells, though the exact cause is not known. [32] Given the improvements in output voltage over the burn-in period and the noted sensitivity of p-i-n monolayer devices to modi cation of the perovskite/C 60 interface, [33,34] this interface may become naturally passivated as the device ages over the initial hours of operation. In sharp contrast, considerable degradation was observed when the perovskite materials were tested in n-i-p devices with spiro-OMeTAD hole transport layers.…”

Section: Operational Stabilitymentioning

confidence: 99%

Operational stability, low light performance, and long-lived transients in mixed-halide perovskite solar cells with a monolayer-based hole extraction layer

Murdey

Ishikura²,

Matsushige

et al. 2022

Solar Energy Materials and Solar Cells

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Perovskite–organic tandem solar cells with indium oxide interconnect

Cited by 272 publications

References 58 publications

Efficient interconnecting layers in monolithic all-perovskite tandem solar cells

Efficient interconnecting layers in monolithic all-perovskite tandem solar cells

Tunable Photovoltaics: Adapting Solar Cell Technologies to Versatile Applications

Operational stability, low light performance, and long-lived transients in mixed-halide perovskite solar cells with a monolayer-based hole extraction layer

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