“…8,9 However, achieving PMA in Co-based Heusler alloys is still challenging due to their typical cubic crystal structures. 10 Nevertheless, interfacial PMA has been achieved in Co 2 FeSi (CFS), 11 Co 2 FeAl 0.5 Si 0.5 (CFAS), 11 Co 2 FeAl (CFA), 12,13 and Co 2 MnSi (CMS) 14,15 Heusler alloys when they are in contact with oxides, heavy metals (HMs), or perpendicular magnetized film/seed layers, respectively. Although a large TMR ratio of 91% has been experimentally demonstrated at room temperature in p-MTJ with a CFA electrode, 16 it is still much lower than that of 217% in CMS/MgO/CMS MTJ with in-plane magnetic anisotropy.…”