2023
DOI: 10.1002/adom.202300142
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Phase‐Coherent Optical Frequency Up‐Conversion with Millimeter‐Size Zn(3‐ptz)2 Metal‐Organic Framework Single Crystals

Abstract: Metal‐organic frameworks (MOFs) have emerged as candidate materials for nonlinear optics due to their enhanced optical and chemical stability in comparison with conventional organic crystals. However, producing large single crystals that support perfect phase matching conditions for frequency conversion is a long‐standing challenge due to the highly metastable conditions in which MOF crystals tend to self‐assemble in solution. By modulating the synthesis and growth conditions, this limitation is overcome to pr… Show more

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Cited by 6 publications
(1 citation statement)
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“…Several MOF structures have been experimentally synthesized and some of them have already shown potential to be used in nonlinear optics [34][35][36][37][38][39][40][41]. A recent publication reports the experimental demonstration of three-wave and four-wave mixing processes using millimeter-scale MOF single crystal with well-defined phase matching properties [42]. The competitive optical nonlinearities of several polycrystalline MOF samples have stimulated the need to develop a robust computational methodology to screen the MOF databases to understand the structure-property relationship to identify and design potential MOF crystals that are promising.…”
Section: Introductionmentioning
confidence: 99%
“…Several MOF structures have been experimentally synthesized and some of them have already shown potential to be used in nonlinear optics [34][35][36][37][38][39][40][41]. A recent publication reports the experimental demonstration of three-wave and four-wave mixing processes using millimeter-scale MOF single crystal with well-defined phase matching properties [42]. The competitive optical nonlinearities of several polycrystalline MOF samples have stimulated the need to develop a robust computational methodology to screen the MOF databases to understand the structure-property relationship to identify and design potential MOF crystals that are promising.…”
Section: Introductionmentioning
confidence: 99%