Photobiocatalysis: More than just an interesting lab curiosity?

Ma, Yunjian; Wang, Yutong; Wu, Bin; Zhou, Jianle; Yang, Shunong; Zhang, Fangyu; Luo, Keyu; Wang, Yonghua; Hollmann, Frank

doi:10.1016/j.checat.2024.101077

Chem Catalysis

2024

DOI: 10.1016/j.checat.2024.101077

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Photobiocatalysis: More than just an interesting lab curiosity?

Yunjian Ma,

Yutong Wang,

Bin Wu

et al.

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2024

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Cited by 2 publications

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Single‐Electron Oxidation Triggered by Visible‐Light‐Excited Enzymes for Asymmetric Biocatalysis

Yu,

Chen,

Huang

2024

Angewandte Chemie

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By integrating enzymatic catalysis with photocatalysis, photoenzymatic catalysis emerges as a powerful strategy to enhance enzyme catalytic capabilities and provide superior stereocontrol in reactions involving reactive intermediates. Repurposing naturally occurring enzymes using visible light is among the most active directions of photoenzymatic catalysis. This Minireview focuses on a cutting‐edge strategy in this direction, namely single‐electron‐oxidation triggered non‐natural biotransformations catalyzed by photoexcited enzymes. These straightforward transformations feature a unique radical mechanism initiated by single‐electron‐oxidation, achieving redox‐neutral non‐natural C‐C, C‐O, and C‐S bond formations, and expanding the chemical toolbox of enzymes. By highlighting recent advances in this field and emphasizing their catalytic mechanisms and synthetic potentials, innovative approaches for further photobiomanufacturing are anticipated.

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Single‐Electron Oxidation Triggered by Visible‐Light‐Excited Enzymes for Asymmetric Biocatalysis

Yu,

Chen,

Huang

2024

Angewandte Chemie

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Single‐Electron Oxidation Triggered by Visible‐Light‐Excited Enzymes for Asymmetric Biocatalysis

Yu,

Chen,

Huang

2024

Angew Chem Int Ed

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Photobiocatalysis: More than just an interesting lab curiosity?

Cited by 2 publications

References 165 publications

Single‐Electron Oxidation Triggered by Visible‐Light‐Excited Enzymes for Asymmetric Biocatalysis

Single‐Electron Oxidation Triggered by Visible‐Light‐Excited Enzymes for Asymmetric Biocatalysis

Single‐Electron Oxidation Triggered by Visible‐Light‐Excited Enzymes for Asymmetric Biocatalysis

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