2024
DOI: 10.1002/ange.202319515
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Photochemische Cobaltkatalysierte Synthese von Heterozyklen durch die Zykloisomerisierung Nichtaktivierter Olefine

Henry Lindner,
Willi M. Amberg,
Tristano Martini
et al.

Abstract: We report a general, intramolecular cycloisomerization of unactivated olefins with pendant nucleophiles. The reaction proceeds under mild conditions and tolerates ethers, esters, protected amines, acetals, pyrazoles, carbamates, and arenes. It is amenable to N‐, O‐, as well as C‐nucleophiles, yielding a number of different heterocycles including, but not limited to, pyrrolidines, piperidines, oxazolidinones, and lactones. Use of both a benzothiazinoquinoxaline as organophotocatalyst and a Co‐salen catalyst obv… Show more

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