2018
DOI: 10.1021/acs.jpca.8b02921
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Photoelectron Spectroscopy of the Aminomethoxide Anion, H2C(NH2)O

Abstract: We report the photoelectron spectrum of the aminomethoxide anion (HC(NH)O). The electron affinity (EA) of the aminomethoxy radical is determined to be 1.944(1) eV. Transitions to the ground (X̃ A″) and first excited (ÃA') electronic states of aminomethoxy are observed, with the term energy measured to be T(Ã ← X̃) = 0.085(1) eV. A long vibrational progression is observed for the transition to the ground X̃ A″ electronic state of aminomethoxy, primarily consisting of OCN bending and HNH wagging vibrations, lead… Show more

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