Photoreduction of carbon dioxide into methane and ethylene using TiO2 inverse opal-derived PCN-222(M)

Liang, Fang-yu; Peng, Yen-Ping; Lin, Kun-Yi Andrew; Huang, Po-Jung

doi:10.1016/j.jece.2024.113825

Journal of Environmental Chemical Engineering

2024

DOI: 10.1016/j.jece.2024.113825

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Photoreduction of carbon dioxide into methane and ethylene using TiO2 inverse opal-derived PCN-222(M)

Fang-yu Liang,

Yen-Ping Peng,

Kun-Yi Andrew Lin

et al.

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Porphyrin-Based Supramolecular Self-Assemblies: Construction, Charge Separation and Transfer, Stability, and Application in Photocatalysis

Hu,

Peng,

Liu

et al. 2024

Molecules

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As a key means to solve energy and environmental problems, photocatalytic technology has made remarkable progress in recent years. Organic semiconductor materials offer structural diversity and tunable energy levels and thus attracted great attention. Among them, porphyrin and its derivatives show great potential in photocatalytic reactions and light therapy due to their unique large-π conjugation structure, high apparent quantum efficiency, tailorable functionality, and excellent biocompatibility. Compared to unassembled porphyrin molecules, supramolecular porphyrin assemblies facilitate the solar light absorption and improve the charge transfer and thus exhibit enhanced photocatalytic performance. Herein, the research progress of porphyrin-based supramolecular assemblies, including the construction, the regulation of charge separation and transfer, stability, and application in photocatalysis, was systematically reviewed. The construction strategy of porphyrin supramolecules, the mechanism of charge separation, and the intrinsic relationship of assembling structure-charge transfer-photocatalytic performance received special attention. Surfactants, peptide molecules, polymers, and metal ions were introduced to improve the stability of the porphyrin assemblies. Donor-acceptor structure and co-catalysts were incorporated to inhibit the recombination of the photoinduced charges. These increase the understanding of the porphyrin supramolecules and provide ideas for the design of high-performance porphyrin-based photocatalysts.

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Porphyrin-Based Supramolecular Self-Assemblies: Construction, Charge Separation and Transfer, Stability, and Application in Photocatalysis

Hu,

Peng,

Liu

et al. 2024

Molecules

View full text Add to dashboard Cite

show abstract

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Photoreduction of carbon dioxide into methane and ethylene using TiO2 inverse opal-derived PCN-222(M)

Cited by 1 publication

References 85 publications

Porphyrin-Based Supramolecular Self-Assemblies: Construction, Charge Separation and Transfer, Stability, and Application in Photocatalysis

Porphyrin-Based Supramolecular Self-Assemblies: Construction, Charge Separation and Transfer, Stability, and Application in Photocatalysis

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