2013
DOI: 10.1088/1674-1056/22/11/114209
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Physical origin of observed nonlinearities in Poly (1-naphthyl methacrylate): Using a single transistor—transistor logic modulated laser beam

Abstract: A thermal lens technique is adopted using a single modulated continuous wave (cw) 532-nm laser beam to evaluate the nonlinear refractive index n 2 , and the thermo-optic coefficient dn/dT , in polymer Poly (1-naphthyl methacrylate) (P-1-NM) dissolved in chloroform, tetrahydrofuran (THF), and dimethyl sulfoxide (DMSO) solvents. The results are compared with Z-scan and diffraction ring techniques. The comparison reveals the effectiveness and the simplicity of the TTL modulation technique. The physical origin is … Show more

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Cited by 20 publications
(3 citation statements)
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“…It is well known that when an intense laser beam passes through a nonlinear Kerr medium, its spatial profile changes as a consequence of lasermatter interaction and after exiting the medium, a set of concentric rings can be observed on a far-field screen. [12,23,24] In Z-scan experiments, the aperture should be placed at the farfield and hence one should always keep in mind the possibility of ring formation on its plane that can alter the amount of radiation which passes through it. Equation (6) represents the integral which is mostly used for interpreting these concentric rings.…”
Section: Resultsmentioning
confidence: 99%
“…It is well known that when an intense laser beam passes through a nonlinear Kerr medium, its spatial profile changes as a consequence of lasermatter interaction and after exiting the medium, a set of concentric rings can be observed on a far-field screen. [12,23,24] In Z-scan experiments, the aperture should be placed at the farfield and hence one should always keep in mind the possibility of ring formation on its plane that can alter the amount of radiation which passes through it. Equation (6) represents the integral which is mostly used for interpreting these concentric rings.…”
Section: Resultsmentioning
confidence: 99%
“…Therefore, a continuous-wave laser beam (653 nm) passing through the sample film can be switched ON and OFF by the TTL modulated beam (473 nm wavelength). [41]. The mechanism covered all-optical switching can be explained as the following: the pumping pulse passes through the sample causes an increase in the population of the triplet states, and thus induces a reduction in the transmittance of the probe beam due to the high absorption of its intensity.…”
Section: All-optical Switchingmentioning
confidence: 99%
“…Currently, the methods available for direct measurement of these two parameters are mentioned in [18], the Z-scan method [19,20] is considered the best because its requirements are simple compared to other methods that require difficult requirements [21,22], its results are very accurate and it has the ability to calculate the real and imaginary parts of the nonlinear optical third-order susceptibility separately. This technique has been used during the last three decades by many researchers to calculate the n 2 and ( ) c 3 of vast number of materials [23][24][25][26][27][28][29][30][31][32][33]. In the indirect measurements the use of the results of the absorption and transmission spectra of the material and theoretical formulas for calculating the nonlinear optical third-order susceptibility and nonlinear index of refraction, also this method was used by researchers in recent years [34][35][36][37][38][39][40][41][42][43].…”
Section: Introductionmentioning
confidence: 99%