and various applications particularly at the microscopic scale. This includes optical trapping and manipulation, [4][5][6] optical telecommunications, [7,8] quantum physics, [9] and "super-resolution" microscopy with a spatial resolution beyond the diffraction limit. [10][11][12] New applications for OAM fields have also been proposed in environmental optics and free-space telecommunication. As an example OAM states can potentially propagate though air turbulence with lower degradation than a conventional Gaussian beam. [13,14] New physical effects include studies such as the rotational Doppler effect originating from interactions of such fields and rotating objects that may provide new technologies for remote sensing of rotating bodies in astrophysics. [15,16] In this area of original physical demonstrations, recent studies have shown that irradiation by such an OAM field can twist materials, such as metal, silicon, azo-polymer, and even a liquid-phase resin with the help of spin angular momentum (SAM) of circularly polarized light with the rotating electric field. This can thus shape helical nano/microstructures. [17][18][19][20][21][22][23][24] Going beyond fundamental aspects, twisted materials created by such OAM fields may provide a new understanding of interactions between optical fields and matter on the subwavelength scale that may reveal new physics, e.g., spin-orbit coupling effects or unconventional optomechanical effects for moving beyond traditional forms of optical manipulation. Furthermore, twisted materials created by such OAM fields, will provide a new understanding of interactions between optical fields and matter on a subwavelength scale. For example, the twisted materials manifest the role of both SAM and OAM of light fields and the coupling of SAM and OAM (so-called spin-orbit coupling) effects. This coupling is key not only for understanding fundamental physics but also for controlling optical material structures.Conventional optical tweezers rely on the field gradients near the diffraction limited focus of a laser beam to hold mesoscopic particles solely with focused light beams. However, the technique often fails to efficiently trap and manipulate particles at the nanoscale because the gradient force scales with the volume of the particle (for a dielectric object) and is proportional to the particle's polarizability. In this domain, advanced materials science and nanofabrication technologies have made remarkable progress in structured devices, e.g., photonic crystals, metamaterials, and metasurfaces. These devices offer novel trapping geometries to enhance the interaction between optical fields and materials at the nanoscale. Furthermore, these devices allow the control of Recent work has shown that irradiation with light possessing orbital angular momentum (OAM) and an associated phase singularity, that is an optical vortex, twists a variety of materials. These include silicon, azo-polymer, and even liquid-phase resins to form various helically structured materials. This article provides...