2018
DOI: 10.1038/s41377-018-0108-8
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Plasmonic mid-infrared third harmonic generation in germanium nanoantennas

Abstract: We demonstrate third harmonic generation in plasmonic antennas consisting of highly doped germanium grown on silicon substrates and designed to be resonant in the mid-infrared frequency range that is inaccessible with conventional nonlinear plasmonic materials. Owing to the near-field enhancement, the result is an ultrafast, subdiffraction, coherent light source with a wavelength tunable between 3 and 5 µm, and ideally overlapping with the fingerprint region of molecular vibrations. To observe the nonlinearity… Show more

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Cited by 51 publications
(26 citation statements)
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“…In 2018, Autore et al took advantage of the large‐quality factors of phonon polaritons in h‐BN nanoribbons to realize molecular vibrational spectroscopy. In addition, subdiffractional nanostructures, which display high confinement of light, can also enhance nonlinear optical effects within these structures …”
Section: Far‐field Optical Methodsmentioning
confidence: 99%
“…In 2018, Autore et al took advantage of the large‐quality factors of phonon polaritons in h‐BN nanoribbons to realize molecular vibrational spectroscopy. In addition, subdiffractional nanostructures, which display high confinement of light, can also enhance nonlinear optical effects within these structures …”
Section: Far‐field Optical Methodsmentioning
confidence: 99%
“…Recently, great scientific effort is devoted towards establishing nanostructures suitable for in-vivo enhanced fluorescence monitoring [4] and surface-enhanced pump-probe schemes to deliver molecular bond information with ultimate sensitivity [7]. Moreover, antennas based on highly-doped semiconductors (HDSCs) have been proposed for third harmonic generation in the mid-infrared [8] since they offer a tunable bulk plasma frequency through doping and high thirdorder susceptibility. This makes them promising candidates for surface-enhanced ultrafast pump-probe vibrational spectroscopy, providing previously inaccessible information about the target molecule and its biological environment.…”
Section: Statusmentioning
confidence: 99%
“…The Ge-on-Si waveguide platform is as an excellent candidate since it could provide low loss guiding from 2 to 15 μm wavelength [3]. This platform has already demonstrated several sensing components in the MIR such as light emitters [4], plasmonic antennas [5], intersubband photodetectors [6] and third harmonic generation [7].…”
Section: Introductionmentioning
confidence: 99%