Polarization-dependent magnetic properties of periodically driven $α$-RuCl$_{3}$

Abstract

We study magnetic properties of a periodically driven Mott insulator with strong spin-orbit coupling and show some properties characteristic of linearly polarized light. We consider a t2g-orbital Hubbard model driven by circularly or linearly polarized light with strong spin-orbit coupling and derive its effective Hamiltonian in the strong-interaction limit for a high-frequency case. We show that linearly polarized light can change not only the magnitudes and signs of the exchange interactions, but also their bond anisotropy even without the bond-anisotropic hopping integrals. Because of this property, the honeycomb-network spin system could be transformed into weakly coupled zigzag or step spin chains for the light field polarized along the b-or a-axis, respectively. Then, analyzing how the light fields affect several magnetic states in a mean-field approximation, we show that linearly polarized light can change the relative stability of the competing magnetic states, whereas such a change is absent for circularly polarized light. We also analyze the effects of both the bond anisotropy of nearest-neighbor hopping integrals and a third-neighbor hopping integral on the magnetic states and show that the results obtained in a simple model, in which the bondaveraged nearest-neighbor hopping integrals are considered, remain qualitatively unchanged except for the stability of zigzag states in the non-driven case and the degeneracy lifting of the zigzag or stripy states.