Free electrons can possess an intrinsic orbital angular momentum, similar to those in an electron cloud, upon free-space propagation. The wavefront corresponding to the electron's wavefunction forms a helical structure with a number of twists given by the angular speed. Beams with a high number of twists are of particular interest because they carry a high magnetic moment about the propagation axis. Among several different techniques, electron holography seems to be a promising approach to shape a conventional electron beam into a helical form with large values of angular momentum. Here, we propose and manufacture a nano-fabricated phase hologram for generating a beam of this kind with an orbital angular momentum up to 200 . Based on a novel technique the value of orbital angular momentum of the generated beam are measured, then compared with simulations. Our work, apart from the technological achievements, may lead to a way of generating electron beams with a high quanta of magnetic moment along the propagation direction, and thus may be used in the study of the magnetic properties of materials and for manipulating nano-particles.Almost a century ago Rutherford and Bohr proposed a model, the so-called Bohr model, to describe the structure of atoms in which model atoms consist of a positive nucleus surrounded by orbiting electrons [1, 2]. Even in this semiclassical model, orbiting electrons possess a quantized orbital motion, i.e. orbital angular momentum (OAM). This quantization, indeed, lies at the heart of the rotationally symmetric nature of the atom. However, it took quite a long time to theoretically predict and experimentally demonstrate that free electrons can also carry a quantized OAM value upon freespace propagation [3][4][5]. The wavefront of electrons carrying a quantized OAM forms a helical shape exp (imϕ) with an integer winding index m, where ϕ is the azimuthal angle in polar coordinates. A free electron with such a helical phasefront possesses an OAM value of m along the propagation direction, and has a magnetic moment µ OAM = mµ B oriented along the beam axis with a polarity that depends on the sign of m. µ B = e /(2m e ) is the Bohr magneton of the electron, is the Planck constant, e and m e are the electron charge and rest mass, respectively. This magnetic moment, unlike the spin Bohr magneton, in principle is unbounded and can be large if desired. Nonetheless, it is bounded by the accuracy of phase modulation and the numerical aperture of the electron optics [6]. The spatial density distribution of these electrons in the transverse plane -orthogonal to propagation directionappears to be a doughnut shape, because a helical phase is undefined at the origin. Moreover, the current density associated with the wavefunction of "twisted" electrons circulates about the origin; thus, these beams are also called electron vortex beams (EVBs). Twisted electron beam (EBs) possess a novel magnetic moment µ OAM along the propagation axis, and thus found immediate applications in the study of materials [7,8]...