2022
DOI: 10.48550/arxiv.2201.10265
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Polaron-enhanced polariton nonlinearity in lead halide perovskites

Abstract: Exciton-polaritons offer a versatile platform for realization of all-optical integrated logic gates due to the strong effective optical nonlinearity resulting from the exciton-exciton interactions. In most of the current excitonic materials there exists a direct connection between the exciton robustness to thermal fluctuations and the strength of exciton-exciton interaction, making materials with highest levels of exciton nonlinearity applicable at cryogenic temperatures only. Here, we show that strong polaron… Show more

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“…Our results are also helpful for resolving the thermal challenges for all-dielectric resonator-based photonic devices [39], Raman microlasers [40,41], and nanoscale photo-thermal chemistry and sensing [42][43][44]. As an outlook, we believe that the developed bistability approach is quite universal and can be further applied not only for various types of nonlinearities based on Kerr effect [45,46], electron-hole plasma generation [32,33,47] and excitonic effects [48][49][50].…”
Section: Discussionmentioning
confidence: 82%
“…Our results are also helpful for resolving the thermal challenges for all-dielectric resonator-based photonic devices [39], Raman microlasers [40,41], and nanoscale photo-thermal chemistry and sensing [42][43][44]. As an outlook, we believe that the developed bistability approach is quite universal and can be further applied not only for various types of nonlinearities based on Kerr effect [45,46], electron-hole plasma generation [32,33,47] and excitonic effects [48][49][50].…”
Section: Discussionmentioning
confidence: 82%