2012
DOI: 10.1021/nn302413u
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Polystyrene Particles Reveal Pore Substructure As They Translocate

Abstract: In this article, we report resistive-pulse sensing experiments with cylindrical track-etched PET pores, which reveal that the diameters of these pores fluctuate along their length. The resistive pulses generated by polymer spheres passing through these pores have a repeatable pattern of large variations corresponding to these diameter changes. We show that this pattern of

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Cited by 69 publications
(137 citation statements)
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“…16,22,23 Figure 2 presents recordings performed with a pore that had an average opening diameter of 770 nm. Each type of particle was studied individually from a suspension in 0.1 M KCl, pH 8 in the presence of Tween 80.…”
Section: Resultsmentioning
confidence: 99%
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“…16,22,23 Figure 2 presents recordings performed with a pore that had an average opening diameter of 770 nm. Each type of particle was studied individually from a suspension in 0.1 M KCl, pH 8 in the presence of Tween 80.…”
Section: Resultsmentioning
confidence: 99%
“…The relative depth of a resistive pulse for a spherical particle can be predicted from the following equation: 6,9,22 ோ ିோ…”
Section: Resultsmentioning
confidence: 99%
See 1 more Smart Citation
“…13,16 Using this model (see SI for more details) we determined the radius r of each particle from the resistive pulse intensity Δ R it produced during the passage through the nanochannel. In Figure 4b, we compare diffusion coefficients D extracted from optical track analysis and the dimension of particles determined electrically.…”
mentioning
confidence: 99%
“…8 Pulse shape is a convolution of pore and particle geometry, and pulse shape reflects pore topography. 9 Pulse width is the residence time within the pore, decreases with particle velocity, 10 and increases with particle-pore interactions, such as adsorption. 11 Particle trajectory through the pore also plays an important role in both pulse width and amplitude.…”
Section: Resistive-pulse Sensing With Out-of-plane Nanoporesmentioning
confidence: 99%