Preferential orientation of anisotropic polythiophene rods toward macroscopic chain ordering

Kitao, Takashi; Legrand, Alexandre; Mori, Taizo; Ariga, Katsuhiko; Uemura, Takashi

doi:10.1039/d2me00204c

Mol. Syst. Des. Eng.

2023

DOI: 10.1039/d2me00204c

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Preferential orientation of anisotropic polythiophene rods toward macroscopic chain ordering

Takashi Kitao

Alexandre Legrand

Taizo Mori

et al.

Abstract: The orientation of polymer chains plays an important role in governing the mechanical, optical, and electronic properties of polymeric materials. Here, we reported on the fabrication of anisotropic polythiophene particles...

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2024

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Precise synthesis and assembly of π-conjugated polymers enabled by metal–organic frameworks

Kitao

2024

Bulletin of the Chemical Society of Japan

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π-conjugated polymers hold considerable promise as key materials in various devices because of their advantageous optical, electronic, and magnetic properties; however, their strong inter-chain π–π interactions render them insoluble without the introduction of solubilizing substituents, making their synthesis highly challenging. Confined synthesis of π-conjugated polymers inside metal–organic frameworks (MOFs) offer a solution to this challenge by isolating the individual polymer chains, effectively addressing solubility issues and regulating polymerization reactions to yield novel π-conjugated polymers that are otherwise inaccessible. This account reviews recent advances in the synthesis and assembly control of π-conjugated polymers within MOFs to enhance physicochemical properties. Additionally, we explore the nanohybridization of π-conjugated polymers with MOFs, leading to sophisticated architectures with intriguing functionalities.

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Precise synthesis and assembly of π-conjugated polymers enabled by metal–organic frameworks

Kitao

2024

Bulletin of the Chemical Society of Japan

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Preferential orientation of anisotropic polythiophene rods toward macroscopic chain ordering

Abstract: The orientation of polymer chains plays an important role in governing the mechanical, optical, and electronic properties of polymeric materials. Here, we reported on the fabrication of anisotropic polythiophene particles...

Cited by 1 publication

References 61 publications

Precise synthesis and assembly of π-conjugated polymers enabled by metal–organic frameworks

Precise synthesis and assembly of π-conjugated polymers enabled by metal–organic frameworks

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