Based on the optimal estimation (OE) theory and information content analysis method, we discuss the ability to include the multi-angle satellite ultraviolet polarization channel to retrieve the aerosol layer height (ALH) for ten typical aerosol types in the China region. We also quantitatively evaluate the effects of polarization measurements and the number of viewing angles on ALH retrieval under different conditions (aerosol model, aerosol optical depth, etc.). By comparing the different degree of freedom for signal (DFS) results of ALH caused by the theoretical retrieval error changes in different microphysical parameters in the aerosol and surface model, we identify the key factors affecting ALH retrieval. The results show that the extended ultraviolet band provides important information for ALH retrieval and is closely related to the scattering and absorption characteristics of aerosol models. The polarization measurements in fine mode reduce the posterior error of ALH retrieval by 6%–39%; however, this is relatively small for coarse mode. In particular, when it is applied to the transported dust and background dust aerosol types, the posterior error is only reduced by 1%–8% after adding polarization measurements. For these two aerosol types with weak absorption at the ultraviolet band, increasing the number of angles observed in addition to increasing the polarization channel will more effectively improve ALH inversion. Compared with other aerosol and surface model parameters, the retrieval errors for the total volume column, effective variance, real part of the complex refractive index, and surface reflectance are the main factors affecting ALH retrieval. Therefore, reducing the theoretical retrieval error of these parameters will be helpful.