The nanosheets TiO 2 /g-C 3 N 4 hybrid material with efficient visible-light photocatalytic activity was prepared by a facile solvothermal method. The as-prepared TiO 2 /g-C 3 N 4 nanosheets composite was thoroughly characterized by X-ray diffraction, Fourier transform infrared spectroscopy, transmission electron microscopy, N 2 adsorption-desorption analysis, UV-Vis diffuse reflectance spectroscopy, and X-ray photoelectron spectroscopy. As evaluated by the degradation of methylene blue under visible light irradiation, TiO 2 /g-C 3 N 4 hybrid composites exhibit much higher photocatalytic activity than pristine g-C 3 N 4 and TiO 2 , respectively. The significant enhancement in photodegradation activity over the TiO 2 /g-C 3 N 4 photocatalyst can be ascribed to the combined effects of the nanosheet structure and subsequent efficient separation of photogenerated charge carriers. A tentative mechanism for the photodegradation process was proposed.