The Arctic is warming two to three times faster than the global average, partly due to changes in short-lived climate forcers (SLCFs) including aerosols. In order to study the effects of atmospheric aerosols in this warming, recent past and future (2015-2050) simulations have been carried out using the GISS-E2.1 Earth system model to study the aerosol burdens and their radiative and climate impacts over the Arctic (>60 °N), using anthropogenic emissions from the Eclipse V6b and the Coupled Model Intercomparison Project Phase 6 (CMIP6) databases. Surface aerosol levels, in particular black carbon (BC) and sulfate (SO4 2-), have been significantly underestimated by more than 50%, with the smallest biases calculated for the nudged atmosphere-only simulations. CMIP6 simulations performed slightly better in simulating both surface concentrations of aerosols and climate parameters, compared to the Eclipse simulations. In addition, fully-coupled simulations had slightly smaller biases in aerosol levels compared to atmosphere only simulations without nudging. Arctic BC, organic carbon (OC) and SO4 2burdens decrease significantly in all simulations following the emission projections, with the CMIP6 ensemble showing larger reductions in Arctic aerosol burdens compared to the Eclipse ensemble. For the 2030-2050 period, both the Eclipse Current Legislation (CLE) and the Maximum Feasible Reduction (MFR) ensembles simulated an aerosol top of the atmosphere (TOA) forcing of -0.39±0.01 W m -2 , of which -0.24±0.01 W m -2 were attributed to the anthropogenic aerosols. The CMIP6 SSP3-7.0 scenario simulated a TOA aerosol forcing of -0.35 W m -2 for the same period, while SSP1-2.6 and SSP2-4.5 scenarios simulated a slightly more negative TOA forcing (-0.40 W m -2 ), of which the anthropogenic aerosols accounted for -0.26 W m -2 . Finally, all simulations showed