It was reported that micrometer-sized ductile crystalline phases can improve the ductility of Zr-based bulk metallic glasses. The present authors reported the synthesis of bulk metallic glass composites by a process combining cooling slope casting and suction casting for Zr66.4Nb6.4Cu10.5Ni8.7Al8alloys. This study aims to investigate basics of Zr-based metallic glass matrix composites with semisolid structure. As a result, it was found that the Zr-based metallic glass matrix composites with very uniform semisolid structure can be produced by heat treatment process at semisolid region. Moreover, it was found that experimental results can be explained by the pseudo-binary phase diagram.