Progress in the understanding of fracture related laser damage of fused silica

Abstract

Numerous experimental and theoretical contributions in the past have stressed the detrimental effect of fractures in the generation of surface laser damage sites in fused silica illuminated at 351 nm. However, two very important steps lack for the moment on the way towards a scientific understanding of the role of fractures. 1. a physical model must be developed to predict damage events starting from real defect sites 2. a reproducible measurement must be obtained and compared with calculations.Here we present the theoretical work realized to reach the first goal. Contrary to previous discussions on fractures, the electromagnetic configuration is calculated in the case of a real material, with electronic surface states, bulk defects, and defects dynamics. Due to electromagnetic field enhancement in the fracture, surface defects absorb a sufficient part of laser energy, able to heat silica above the vaporization temperature. This is the initial event that triggers production of more excited states during the pulse, and steep increase of temperature and pressure fields. Comparisons with available experimental results are positive. Calculated fluences of damage initiation are very near those of measured events on engineered fractures, or on real defects in polished samples.

Effects of wavelengths combination on initiation and growth of laser-induced surface damage in SiO 2

“…In order to quantify this effect, we fit data from These values are only an indication of the 1w contribution. They have to be confirmed by numerical simulations [6]. According to Demos et al [7], the presence of a plasma is correlated with the growth phenomenon.…”

Fracture related initiation and growth of surface laser damage in fused silica

“…Hence, a fracture surface involving quantum states in the forbidden band can play this role. 1 Several experiments suggest that surfaces are involved in laser energy absorption by dielectric materials, 5,6 more precisely a surface layer within the nanometer scale. 7 Accordingly, we introduce in our model such an absorbing layer ( Fig.…”

Loose abrasive slurries for optical glass lapping

“…Various authors have shown that residual subsurface cracks existing in fused silica optics are likely to be precursors of laser damage [3][4][5][6]. Hence, efforts have been made by us and many others to measure and understand the impact of each manufacturing process step on the creation of subsurface damage (SSD) under the final fused silica surface [7][8][9][10][11].…”