The concentric pushing method was used to study the bonding properties between polymer and concrete. This paper studied the influence of polymer density, environmental temperature, and moisture content of concrete between polymer and concrete on the bond strength. The results indicated that the bond failure of specimens occurred mainly when the polymer was pushed out. Furthermore, increasing the polymer density increases the bond strength at the polymer-concrete interface but decreases as the moisture content of the concrete increases. The environmental temperature affects the curing time, and the bond strength increases with increasing temperature. Under the same condition, the bond strength was influenced by the roughness of the interface. This study provides references for the construction design and enhances polymer materials and matrix application for repairing cracks in concrete dams.