“…[1±3] In the last few years, solid-state SRS science and technology were becoming more widespread. [4,5] Growth in the activity has been made possible by the discovery of several new SRS active crystals (examples, see the literature [6±10] ), including a successful application given by nano-and picosecond Raman lasers generating specific and otherwise hard to reach wavelengths in a wide spectral range, covering also the eye-safe area. [11±16] Among other technological applications of new Raman lasers, remote sensing of the atmosphere is of great interest, which typically requires high peak-power laser pulses at wavelengths that are difficult to produce by other all-solid-state laser systems.…”