This work presents a unique technique for optimising composite laminates used as structural components, which is critical for situations where failure might result in disastrous effects. Unlike traditional surrogate‐based optimisation approaches, this methodology combines the accurate modelling capabilities of finite element (FE) analysis with the iterative refining capacity of metaheuristic algorithms. By combining these two methodologies, our method intends to improve the design process of laminated shell structures, assuring robustness and dependability is crucial. Compared to existing benchmark solutions, the current FE shows a <1% error for cylindrical and spherical shells. The prime objective of this study is to identify the optimum ply angles for attaining a high fundamental frequency. The problem is NP‐hard because the possible ply angles span a wide range (±90°), making it difficult for optimisation algorithms to find a solution. Seven popular metaheuristic algorithms, namely the genetic algorithm (GA), the ant lion optimisation (ALO), the arithmetic optimisation algorithm (AOA), the dragonfly algorithm (DA), the grey wolf optimisation (GWO), the salp swarm optimisation (SSO), and the whale optimisation algorithm (WOA), are applied to and compared on a wide range of shell design problems. It assesses parameter sensitivity, discovering significant design elements that influence dynamic behaviour. Convergence studies demonstrate the superior performance of AOA, GWO, and WOA optimisers. Rigorous statistical comparisons assist practitioners in picking the best optimisation technique. FE‐GWO, FE‐DA, and FE‐SSA methods surpass the other techniques as well as the layerwise optimisation strategy. The findings obtained, employing the GWO, DA, and SSA optimisers, demonstrate ~3% improvement over the existing literature. With respect to conventional layup designs (cross‐ply and angle‐ply), the current optimised designs are better by at least 0.43% and as much as 48.91%.