“…In the past years, some attempts to improve the mechanical properties have been done by the addition of oxide particles like ZrO 2 , MgO, and Bi 4 Ti 3 O 12 [3][4][5], but the piezoelectric constant d 33 and the electromechanical coupling factor K P decreased dramatically. Recently, significant improvement of mechanical properties, corresponding with a slightly sacrificed value of d 33 , was achieved in PZT/ZrO 2 , PZT/MgO and PZT/ZnO composites [6][7][8], while the problem of the deterioration of K P still remains unsolved.…”