The impact of anti-site disorder x on the intrinsic Gilbert damping α 0 in well-ordered 1 FePt films is investigated by time-resolved magneto-optical Kerr effect. The variation of x mainly affects the electron scattering rate 1/τ e , while other leading parameters remain unchanged. The experimentally observed linear dependence of α 0 on 1/τ e indicates that spin relaxation is through electron interband transitions, as predicted by spin-orbit coupling torque correlation model. Measurements at low temperature show that α 0 remains unchanged with temperature even for FePt with very high chemical order, indicating that electron-phonon scattering is negligible. Moreover, as x decreases the perpendicular magnetic anisotropy increases and the Landau g factor exhibits a negative shift due to an increase in orbital momentum anisotropy. Our results will facilitate the design and exploration of new magnetic alloys with large magnetic anisotropy and desirable damping properties.PACS numbers: 75.78. Jp, 75.70.Tj, 75.50.Vv, 75.30.Gw + e-mail: hbzhao@fudan.edu.cn *e-mail: gxluep@wm.edu.[2]
IntroductionUltrafast magnetization precessional switching in ferromagnets utilizing magnetic field pulses, spin polarized currents, and ultrafast laser pulses [1][2][3][4][5][6] is currently a popular topic due to its importance in magnetic information storage and spintronic applications. The uniform magnetization precession can be well modeled with Landau-Lifshitz-GilbertSlonczewski (LLGS) equation [7][8][9], where the Slonczewski torque term denotes the spin transfer torques (STTs), and the Gilbert damping parameter α determines the spin relaxation time [10] and is crucial for device performance [11][12][13][14]. The extrinsic Gilbert damping is due to nonlocal spin relaxation, such as spin pumping and magnon-magnon scattering, which can be tuned by artificial substrates, specially designed buffer and coverage layers [15][16][17][18][19][20][21], while the intrinsic Gilbert damping parameter α 0 is thought to arise from spin-orbit interaction (SOI) [22][23][24][25][26][27][28][29][30], and recently its quadratic dependence on SOI is demonstrated experimentally in FePtPd alloys [31].The α 0 describes the energy flow rate from spin to electronic orbital and phonon degrees of freedom through electron scattering, and has been studied in various theoretical models [22][23][24][25][26][27][28][29][30]. The breathing Fermi surface model [22] and torque-correlation model [23] based on first principle band structure calculations qualitatively match α 0 in soft magnetic alloys such as Fe, . Moreover, contributions to α 0 can be categorized based on intraband and interband transitions [23,26]. The damping rate from intraband transitions scales linearly with the electron relaxation time τ e and exhibits conductivity-like behavior. In contrast, the damping rate from the interband transition is proportional to the electron scattering rate 1/τ e , and consequently exhibits resistivity-like behavior. Therefore, the transition from conductivity-like to re...