2021
DOI: 10.1364/ol.418398
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Quantum-enhanced two-photon spectroscopy using two-mode squeezed light

Abstract: We investigate the prospects of using two-mode intensity squeezed twin beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof-of-principle demonstration, we recorded quantum-enhanced measurements of the Rb 5 D 3 / 2 hyperfine structure with reduced requirements for the Raman pump laser power and Rb vapor number density.

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Cited by 29 publications
(7 citation statements)
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“…A long-term goal of the investigation non-classical light is to actually take advantage of the noise or correlation properties in measurements in a system that can potentially be moved out of the lab [159]. A number of specific demonstrations of the use of squeezed light generated in hot vapors have been made, including in plasmonic sensors [160,161], two-photon spectroscopy [162], cantilever sensors in atomic force microscopy [163], interferometry [164][165][166], and especially magnetometry [25,167]. The enhancement of two-photon absorption using twin-beam sources of correlated light for the possible improvement of the sensitivity of two-photon microscopy is also a current topic of interest [168].…”
Section: Discussionmentioning
confidence: 99%
“…A long-term goal of the investigation non-classical light is to actually take advantage of the noise or correlation properties in measurements in a system that can potentially be moved out of the lab [159]. A number of specific demonstrations of the use of squeezed light generated in hot vapors have been made, including in plasmonic sensors [160,161], two-photon spectroscopy [162], cantilever sensors in atomic force microscopy [163], interferometry [164][165][166], and especially magnetometry [25,167]. The enhancement of two-photon absorption using twin-beam sources of correlated light for the possible improvement of the sensitivity of two-photon microscopy is also a current topic of interest [168].…”
Section: Discussionmentioning
confidence: 99%
“…where θ is the phase of the homodyne detector. The optimized squeezing depth over the phases θ turns out to be [42] Using equations ( 37)-( 40), S opt for the output state in equation ( 11) is plotted in figure 12. Special case, when m = 0, we have S opt = 0, which means no squeezing as expected.…”
Section: Squeezing-enhanced Coherent Statementioning
confidence: 99%
“…[35,36], which noted that interactions can enable socalled "super-Heisenberg scaling" with the photon number n in the sense that the optimal scaling of linear phase estimation precision (∼n −1 ) can be surpassed. These studies concern linear spectroscopy, i.e., the absorption of single photons, or the combination of classical lasers with quantum light sources in two-photon Raman transitions [37,38]. The first theoretical works also started to investigate the role of quantum correlations in TPA of entangled photon pairs [39,40] or of photon statistics in coherent control [41].…”
Section: Introductionmentioning
confidence: 99%