Rational design of Ag nanowires growth engineered conductivity chain toward Li/CFx primary batteries with high-energy and high-power density

Wang, Jian; Liu, Yifan; Qin, Guilu; Wu, BaoShan; Yan, Zongkai; Mahmood, Nasir; Jian, Xian; Liu, Huakun

doi:10.1016/j.mtener.2023.101403

Materials Today Energy

2023

DOI: 10.1016/j.mtener.2023.101403

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Rational design of Ag nanowires growth engineered conductivity chain toward Li/CFx primary batteries with high-energy and high-power density

Jian Wang,

Yifan Liu,

Guilu Qin

et al.

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Cited by 3 publications

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Porous Hollow Carbon Alkali-Activated Nanoonions As a Conductive Additive for High-Rate Lithium Primary Batteries

Qin,

Liu,

et al. 2024

ACS Appl. Energy Mater.

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Porous Hollow Carbon Alkali-Activated Nanoonions As a Conductive Additive for High-Rate Lithium Primary Batteries

Qin,

Liu,

et al. 2024

ACS Appl. Energy Mater.

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Elucidating the effects of the carbon source on fluorination kinetics and the CF_x structure to tailor the energy density of Li/CF_x

Zhang,

Li,

et al. 2025

J. Mater. Chem. A

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Three-Dimensional Lithium Anode with an In Situ Generated Li2O-Rich Solid Electrolyte Interface for High-Rate and Long-Storage Lithium Battery

Li,

Liu,

Zhou

et al. 2024

Energies

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The limited rate performance of Li||CFx batteries hinders their wide application, owing to the low conductivity of CFx cathode material and the undesirable solid electrolyte interface (SEI) layer formed on the Li anode surface. Herein, a strategy for constructing a three-dimensional lithium anode (3D-Li anode) with high specific surface area and an in situ formed favorable SEI layer is proposed to enhance the interfacial stability and uniformity of ion transport and realize a Li||CFx battery with remarkable comprehensive performance. A 3D-Li anode (Li@CuO-Cu foam) is successfully constructed by molten Li infusion of a thermal oxidation processed copper foam. The lithiophilicity of the Cu foam framework is optimized by the formed CuO. The Li@CuO-Cu foam||CFx battery exhibits a high discharge specific capacity (1149.6 mAh g−1 at 0.1 C) along with a high discharge plateau voltage (2.65 V). At a high rate of 10 C, the 3D-Li anode-based batteries still demonstrate a discharge specific capacity of 463 mAh g−1, which is about 2.5 times that of the conventional Li||CFx, and exhibit excellent storage performance (620.3 mAh g−1 after storage at 55 °C for 90 days) and a low monthly self-discharge rate (1.28%). This work demonstrates a promising strategy to construct a three-dimensional lithium metal anode and significantly improve the rate and storage performance of Li||CFx batteries.

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Rational design of Ag nanowires growth engineered conductivity chain toward Li/CFx primary batteries with high-energy and high-power density

Cited by 3 publications

References 48 publications

Porous Hollow Carbon Alkali-Activated Nanoonions As a Conductive Additive for High-Rate Lithium Primary Batteries

Porous Hollow Carbon Alkali-Activated Nanoonions As a Conductive Additive for High-Rate Lithium Primary Batteries

Elucidating the effects of the carbon source on fluorination kinetics and the CF_x structure to tailor the energy density of Li/CF_x

Three-Dimensional Lithium Anode with an In Situ Generated Li2O-Rich Solid Electrolyte Interface for High-Rate and Long-Storage Lithium Battery

Contact Info

Product

Resources

About

Rational design of Ag nanowires growth engineered conductivity chain toward Li/CFx primary batteries with high-energy and high-power density

Cited by 3 publications

References 48 publications

Porous Hollow Carbon Alkali-Activated Nanoonions As a Conductive Additive for High-Rate Lithium Primary Batteries

Porous Hollow Carbon Alkali-Activated Nanoonions As a Conductive Additive for High-Rate Lithium Primary Batteries

Elucidating the effects of the carbon source on fluorination kinetics and the CFx structure to tailor the energy density of Li/CFx

Three-Dimensional Lithium Anode with an In Situ Generated Li2O-Rich Solid Electrolyte Interface for High-Rate and Long-Storage Lithium Battery

Contact Info

Product

Resources

About

Elucidating the effects of the carbon source on fluorination kinetics and the CF_x structure to tailor the energy density of Li/CF_x