Abstract:Unit‐cell‐thin zeolitic nanosheets have emerged as fascinating materials for catalysis and separation. The controllability of nanosheet stacking is extremely challenging in the chemistry of two‐dimensional zeolitic materials. To date, the organization of zeolitic nanosheets in hydrothermal synthesis has been limited by the lack of tunable control over the guest–host interactions between organic structure‐directing agents (OSDAs) and zeolitic nanosheets. A direct synthetic methodology is reported that enables s… Show more
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