“…Investigations of the nonlinear responses of two-dimensional materials to the light beams have geared up in recent years due to immense applications in optoelectronics like optical switching [1,2], signal processing [3], optical transistors [4], modulators [5], slow light devices [6] and logic gates [7,8]. In particular, research has focused on photovoltaic [9], secondharmonic [10][11][12], third-harmonic [13,14], circular photogalvanic effects [15], etc for time-reversal and inversion symmetric systems [16]. Moreover, the third-order nonlinear optical effects have also been studied in nanostructured systems using the two-wave mixing process considering the first and second harmonic beams [17].…”