2020
DOI: 10.1039/d0ma00384k
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Recent advances in carbon-based supercapacitors

Abstract:

The rapid advancement of modern electronics starves for further breakthroughs to achieve high-energy, large-power and long-running energy-storage devices. Carbon-based supercapacitors (CSs) are promising large-power systems that store electrical energy at...

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Cited by 252 publications
(109 citation statements)
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“…Generally, carbon based materials such as graphene, carbon black, graphene oxide and reduced graphene oxide, etc, exhibit EDLC-type behaviour. In the case of pseudocapacitors, very high energy density is obtained where the charge storage mechanism is probed by fast faradaic redox reactions 5,6 . Different types of metal oxides including spinel 7,8 , transition metal oxides 9,10 and conducting polymers 11,12 have been reported as pseudocapacitive materials.…”
Section: Introductionmentioning
confidence: 99%
“…Generally, carbon based materials such as graphene, carbon black, graphene oxide and reduced graphene oxide, etc, exhibit EDLC-type behaviour. In the case of pseudocapacitors, very high energy density is obtained where the charge storage mechanism is probed by fast faradaic redox reactions 5,6 . Different types of metal oxides including spinel 7,8 , transition metal oxides 9,10 and conducting polymers 11,12 have been reported as pseudocapacitive materials.…”
Section: Introductionmentioning
confidence: 99%
“…24 The metal oxide/carbon composites have been fabricated including carbon nanotubes, carbon nanofibers, graphene, and amorphous carbon materials, which dramatically improved the electroconductivity and further enhanced the specific capacitance and rate performances of the metal oxide/carbon composites. [25][26][27][28][29][30] In this work, cobalt oxide slurry was prepared using cobalt oxide and sucrose, sucrose was used as a soluble carbon source in the slurry. Sucrose has converted into conducting carbon during annealing and coated on cobalt oxide particles.…”
Section: Introductionmentioning
confidence: 99%
“…In this study, we designed a novel gel electrolyte, namely “DMSO/water in salt”‐based chitosan hydrogel electrolyte (DWIS‐CH), using chitosan as the support, H 2 O and DMSO as the solvents, and high concentrations of LiTFSI as the salt [19] . Water molecules can either bind to hydrophilic groups (hydroxy and amino groups) in the hydrogel or interact with Li + to construct a unique 3D ion channel [20] . Compatible with this hydrogel electrolyte, we also prepared an ideal nitrogen‐doped graphene (NG) hydrogel electrode with a large specific surface area through a hydrothermal method.…”
Section: Introductionmentioning
confidence: 99%
“…[19] Water molecules can either bind to hydrophilic groups (hydroxy and amino groups) in the hydrogel or interact with Li + to construct a unique 3D ion channel. [20] Compatible with this hydrogel electrolyte, we also prepared an ideal nitrogen-doped graphene (NG) hydrogel electrode with a large specific surface area through a hydrothermal method. Impressively, the desired allsolid-state hydrogel supercapacitor can be fabricated by means of in situ cross-linking due to the supramolecular complexation between chitosan and Li + -solvated complexes with an appropriate concentration (from 4 to 7 mol L À 1 ).…”
Section: Introductionmentioning
confidence: 99%