2022
DOI: 10.3390/inorganics11010016
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Recent Advances in In Situ/Operando Surface/Interface Characterization Techniques for the Study of Artificial Photosynthesis

Abstract: (Photo-)electrocatalytic artificial photosynthesis driven by electrical and/or solar energy that converts water (H2O) and carbon dioxide (CO2) into hydrogen (H2), carbohydrates and oxygen (O2), has proven to be a promising and effective route for producing clean alternatives to fossil fuels, as well as for storing intermittent renewable energy, and thus to solve the energy crisis and climate change issues that we are facing today. Basic (photo-)electrocatalysis consists of three main processes: (1) light absor… Show more

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Cited by 7 publications
(3 citation statements)
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“…2.4 Å, which is consistent with Ru−Ru bonds of metallic Ru. These operando characterizations were applied to the study of the changes in catalyst surfaces/interfaces [58][59][60]. Except for Pt-group elements as shown in Figure 1d, nonprecious TMs are also ideal substituted catalysts with lower cost.…”
Section: Design Principles Of Cathode and Anodementioning
confidence: 99%
“…2.4 Å, which is consistent with Ru−Ru bonds of metallic Ru. These operando characterizations were applied to the study of the changes in catalyst surfaces/interfaces [58][59][60]. Except for Pt-group elements as shown in Figure 1d, nonprecious TMs are also ideal substituted catalysts with lower cost.…”
Section: Design Principles Of Cathode and Anodementioning
confidence: 99%
“…EXAFS provides insights into bond lengths, coordination numbers, and the presence of defects or disorder, all of which profoundly influence the electronic properties of the heterojunction. 30 Moreover, reverse double-beam photoacoustic spectroscopy (RDB-PAS) proves to be exceptionally useful in the study of charge carrier dynamics within semiconductor heterojunctions. It can provide a detailed picture of the electronic and acoustic responses at the heterojunction interface, crucial for understanding the efficiency and kinetics of charge carriers, which are pivotal factors in the performance of semiconductor heterojunctions, particularly those involved in energy conversion applications.…”
Section: Introductionmentioning
confidence: 99%
“…Extended X-ray absorption fine structure (EXAFS) analysis enables us to investigate the local atomic structure and bonding environment of specific elements within the heterojunction. EXAFS provides insights into bond lengths, coordination numbers, and the presence of defects or disorder, all of which profoundly influence the electronic properties of the heterojunction . Moreover, reverse double-beam photoacoustic spectroscopy (RDB-PAS) proves to be exceptionally useful in the study of charge carrier dynamics within semiconductor heterojunctions.…”
Section: Introductionmentioning
confidence: 99%