2014
DOI: 10.1021/cs500070x
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Recent Development of Molybdenum Sulfides as Advanced Electrocatalysts for Hydrogen Evolution Reaction

Abstract: Hydrogen is expected to play a major role in the development of sustainable energy and environment. Electrocatalytic hydrogen evolution reaction (HER) is known as an efficient method for large-scale hydrogen production, and in this electrochemical process, efficient and low-cost electrocatalysts are indispensable. Recent advances have revealed that nanostructured molybdenum sulfides (MoSx) would be promising alternatives to Pt for the electrochemical generation of hydrogen from water. In this review, we focus … Show more

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Cited by 812 publications
(519 citation statements)
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“…10,11 Since the original studies of Hinneman et al and Jaramillo et al, extensive efforts have been devoted to the preparation of nanostructured crystalline molybdenum sulfide materials for HER; these efforts have been reviewed by us and others. [12][13][14][15] This account deals with a related but different type of molybdenum sulfides -the amorphous materials.…”
Section: Introductionmentioning
confidence: 99%
“…10,11 Since the original studies of Hinneman et al and Jaramillo et al, extensive efforts have been devoted to the preparation of nanostructured crystalline molybdenum sulfide materials for HER; these efforts have been reviewed by us and others. [12][13][14][15] This account deals with a related but different type of molybdenum sulfides -the amorphous materials.…”
Section: Introductionmentioning
confidence: 99%
“…For example, cobalt, [11][12][13] nickel, 14 copper [15][16][17] bimetallic catalyst, 18 transition metal carbide nanocrystals M3C (M: Fe, Co, Ni) encapsulated with vertically aligned graphene nanoribbons, 19 nitrogen and sulfur co-doped nanoporous graphene, 20 molybdenum sulfide (MoS 2 ), phosphide, carbon and noble metal-free catalysts are reported for the HER process. [21][22][23][24] Currently, nanoporous gold films (NPGF) have attracted attention for their widespread application in catalysis and in the sensors field because of their higher surface area in comparison to bulk gold electrodes, allowing superior electron transfer rate between the electrode-electrolyte interface. 25,26 Such platforms have been mainly prepared by alloying/dealloying or template methods, where hazardous chemicals are mostly used.…”
Section: Introductionmentioning
confidence: 99%
“…Accordingly, MoS 2 has been produced in different nanostructured forms such as nanoparticles, defective nanosheets, porous films, nanowires, and amorphous films [37,61,63]. Furthermore, covalent functionalization of the 1T-MoS 2 monolayer modifies its electronic structure, thus allowing an ad hoc tuning of the d-band centre [61].…”
Section: Pt Alloysmentioning
confidence: 99%