“…Since isolated Pt atoms were first anchored on iron oxide to construct Pt 1 /FeO x for CO oxidation, 3 single-atom catalysts (SACs) have attracted extensive attention because of their maximized metal utilization efficiency and extremely high catalytic activity, [4][5][6] especially single metal-doped non-metal coordinated graphene SACs. 7 Moreover, N, O, and S are common coordinated elements in available studies. [8][9][10] However, single metal-doped nitrogen-coordinated graphene (M-N-G) SACs can not only maintain the planar structure of graphene but also effectively regulate the electronic structure of the M atom due to the higher electronegativity of the N atom and a similar atomic size to C, 11 exhibiting good structural stabilities and catalytic activities.…”