Recent progress of two-dimensional metal-base catalysts in urea oxidation reaction

Huang, Qi-Xiang; Wang, Fang; Liu, Yong; Zhang, Bi-Ying; Guo, Fang-Ya; Jia, Zhong-Qiu; Wang, Hao; Yang, Tian-Xiang; Wu, Hai-Tao; Ren, Feng-Zhang; Yi, Ting-Feng

doi:10.1007/s12598-024-02668-y

Rare Met.

2024

DOI: 10.1007/s12598-024-02668-y

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Recent progress of two-dimensional metal-base catalysts in urea oxidation reaction

Qi-Xiang Huang,

Fang Wang,

Yong Liu

et al.

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2024

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Cited by 3 publications

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Ni-based electrocatalysts for urea oxidation reaction: Mechanistic insights and recent advancements

Li,

Zheng,

Guo

et al. 2024

Journal of Alloys and Compounds

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Ni-based electrocatalysts for urea oxidation reaction: Mechanistic insights and recent advancements

Li,

Zheng,

Guo

et al. 2024

Journal of Alloys and Compounds

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Coupled electrocatalytic hydrogen production

Li,

Xu,

Jiang

et al. 2024

Materials Science and Engineering: R: Reports

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Suitable Stereoscopic Configuration of Electrolyte Additive Enabling Highly Reversible and High—Rate Zn Anodes

Xu,

Liu,

Zhao

et al. 2024

Molecules

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Electrolyte additive engineering is a crucial method for enhancing the performance of aqueous zinc—ion batteries (AZIBs). Recently, most research predominantly focuses on the role of functional groups in regulating electrolytes, often overlooking the impact of molecule stereoscopic configuration. Herein, two isomeric sugar alcohols, mannitol and sorbitol, are employed as electrolyte additives to investigate the impact of the stereoscopic configuration of additives on the ZnSO4 electrolyte. Experimental analysis and theoretical calculations reveal that the primary factor for improving Zn anode performance is the regulation of the solvation sheath by these additives. Among the isomers, mannitol exhibits stronger binding energies with Zn2+ ions and water molecules due to its more suitable stereoscopic configuration. These enhanced bindings allow mannitol to coordinate with Zn2+, contributing to solvation structure formation and reducing the active H2O molecules in the bulk electrolyte, resulting in suppressed parasitic reactions and inhibited dendritic growth. As a result, the zinc electrodes in mannitol—modified electrolyte exhibit excellent cycling stability of 1600 h at 1 mA cm−2 and 900 h at 10 mA cm−2, respectively. Hence, this study provides novel insights into the importance of suitable stereoscopic molecule configurations in the design of electrolyte additives for highly reversible and high—rate Zn anodes.

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Recent progress of two-dimensional metal-base catalysts in urea oxidation reaction

Cited by 3 publications

References 131 publications

Ni-based electrocatalysts for urea oxidation reaction: Mechanistic insights and recent advancements

Ni-based electrocatalysts for urea oxidation reaction: Mechanistic insights and recent advancements

Coupled electrocatalytic hydrogen production

Suitable Stereoscopic Configuration of Electrolyte Additive Enabling Highly Reversible and High—Rate Zn Anodes

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