“…[ 49 , 62 , 63 , 64 , 65 , 66 , 67 ] In addition, the interaction of lattice, orbitals, charges, and spins at the heterogeneous interface produces peculiar physical properties, such as “improper ferroelectricity” in short‐period superlattices, ordered vortex arrays in mid‐period superlattices, and flux‐closed domain structures in large‐period superlattices. [ 68 , 69 , 70 , 71 , 72 , 73 ] These phenomena are important for researchers to understand the involved physical phenomena. The influence of this novel properties on the energy storage characteristics of multilayer dielectric needs to be explored.…”